Online ISSN: 1521-3773 Print ISSN: 1433-7851
Angewandte Chemie International Edition
Volume
40, Issue
24,
2001.
© 2001 WILEY-VCH Verlag GmbH, Weinheim, Fed. Rep. of Germany
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Online ISSN: 1521-3773 Print ISSN: 1433-7851 © 2001 WILEY-VCH Verlag GmbH, Weinheim, Fed. Rep. of Germany |
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Cover Picture Jurry M. Hannink, Jeroen J. L. M. Cornelissen, Joan A. Farrera, Philippe Foubert, Frans C. De Schryver, Nico A. J. M. Sommerdijk, Roeland J. M. Nolte Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4519::AID-ANIE4519>3.0.CO;2-# |
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| Graphical Abstract | ||
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Graphical Abstract Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4521::AID-ANIE4521>3.0.CO;2-8 |
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| Corrigendum | ||
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On the Beneficial Effect of ortho-Methoxy Groups in the Asymmetric Ring Opening of meso Epoxides with Silicon Tetrachloride Catalyzed by Chiral ortho-Methoxyphenyldiazaphosphonamide Lewis Bases Gérard Buono Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4536::AID-ANIE4536>3.0.CO;2-D |
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A Lewis Acid Catalyst Anchored on Silica Grafted with Quaternary Alkylammonium Chloride Moieties Thundi M. Jyothi, Mark L. Kaliya, Miron V. Landau Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4536::AID-ANIE11114536>3.0.CO;2-5 |
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| Review | ||
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The B-Alkyl Suzuki-Miyaura Cross-Coupling Reaction: Development, Mechanistic Study, and Applications in Natural Product Synthesis Sherry R. Chemler, Dirk Trauner, Samuel J. Danishefsky Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4544::AID-ANIE4544>3.0.CO;2-N |
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Oxygen Binding, Activation, and Reduction to Water by Copper Proteins Edward I. Solomon, Peng Chen, Markus Metz, Sang-Kyu Lee, Amy E. Palmer Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4570::AID-ANIE4570>3.0.CO;2-4 |
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| Minireview | ||
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Enantioselective Construction of Quaternary Stereocenters Jens Christoffers, Alexander Mann Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4591::AID-ANIE4591>3.0.CO;2-V |
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| Essay | ||
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Coping with Fritz Haber's Somber Literary Shadow Roald Hoffmann, Pierre Laszlo Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4599::AID-ANIE4599>3.0.CO;2-K |
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The Rocky Road to Literary Fame: Marcel Proust and the Diamond Synthesis of Professor Moissan Otto Krätz Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4604::AID-ANIE4604>3.0.CO;2-P |
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| Highlight | ||
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Ru- and Rh-Catalyzed Asymmetric Hydrogenations: Recent Surprises from an Old Reaction Kai Rossen Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4611::AID-ANIE4611>3.0.CO;2-4 |
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| Correspondence | ||
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Comment on the Communication The Key to Solving the Protein-Folding Problem Lies in an Accurate Description of the Denatured State by van Gunsteren et al. Aaron R. Dinner, Martin Karplus Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4615::AID-ANIE4615>3.0.CO;2-H |
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Reply Wilfred F. van Gunsteren, Roland Bürgi, Christine Peter, Xavier Daura Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4616::AID-ANIE4616>3.0.CO;2-B |
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| Communication | ||
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A Trifunctional Catalyst for the Synthesis of Chiral Diols Boyapati M. Choudary, Naidu S. Chowdari, Sateesh Madhi, Mannepalli L. Kantam Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4619::AID-ANIE4619>3.0.CO;2-U |
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TlF and PbO under High Pressure: Unexpected Persistence of the Stereochemically Active Electron Pair Ulrich Häussermann, Pedro Berastegui, Stefan Carlson, Julien Haines, Jean-Michel Léger Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4624::AID-ANIE4624>3.0.CO;2-L |
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Solid-Phase Synthesis of Transition Metal Linked, Branched Oligonucleotides Ignacio Vargas-Baca, Debbie Mitra, Holly J. Zulyniak, Jay Banerjee, Hanadi F. Sleiman Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4629::AID-ANIE4629>3.0.CO;2-S |
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The Mechanism of Hydroamination of Allenes, Alkynes, and Alkenes Catalyzed by Cyclopentadienyltitanium-Imido Complexes: A Density Functional Study Bernd F. Straub, Robert G. Bergman Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4632::AID-ANIE4632>3.0.CO;2-V |
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Self-Assembly of Cyclic Peptides into Nanotubes and Then into Highly Anisotropic Crystalline Materials David Gauthier, Pierre Baillargeon, Marc Drouin, Yves L. Dory Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4635::AID-ANIE4635>3.0.CO;2-D |
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Single-Step, Highly Active, and Highly Selective Nanoparticle Catalysts for the Hydrogenation of Key Organic Compounds Robert Raja, Tetyana Khimyak, John Meurig Thomas, Sophie Hermans, Brian F. G. Johnson Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4638::AID-ANIE4638>3.0.CO;2-W |
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Influence of Structural and Rotational Isomerism on the Triplet Blinking of Individual Dendrimer Molecules Tom Vosch, Johan Hofkens, Mircea Cotlet, Fabian Köhn, Hideki Fujiwara, Roel Gronheid, Koen Van Der Biest, Tanja Weil, Andreas Herrmann, Klaus Müllen, Shaul Mukamel, Mark Van der Auweraer, Frans C. De Schryver Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4643::AID-ANIE4643>3.0.CO;2-N |
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Hydrophobic Groups Stabilize the Hydration Shell of 2-O-Methylated RNA Duplexes Pascal Auffinger, Eric Westhof Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4648::AID-ANIE4648>3.0.CO;2-U |
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Formation and Stabilization of a Decanuclear CuII Wheel Linked by Chloride and OH-N Hydrogen Bonds Che-Hao Chang, Kuo Chu Hwang, Chao-Shiuan Liu, Yun Chi, Arthur J. Carty, Ludmila Scoles, Shie-Ming Peng, Gene-Hsiang Lee, Jan Reedijk Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4651::AID-ANIE4651>3.0.CO;2-X |
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Structure, Immunogenicity, and Protectivity Relationship for the 1585 Malarial Peptide and Its Substitution Analogues Fabiola Espejo, Marcia Cubillos, Luz Mary Salazar, Fanny Guzman, Mauricio Urquiza, Marisol Ocampo, Yolanda Silva, Raul Rodriguez, Eduardo Lioy, Manuel Elkin Patarroyo Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4654::AID-ANIE4654>3.0.CO;2-F |
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-Fibrillogenesis from Rigid-Rod -Barrels: Hierarchical Preorganization Beyond Microns Gopal Das, Lahoussine Ouali, Marc Adrian, Bodo Baumeister, Kevin J. Wilkinson, Stefan Matile Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4657::AID-ANIE4657>3.0.CO;2-Y |
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Construction of Carbon Nanotube Stars with Dendrimers Masahito Sano, Ayumi Kamino, Seiji Shinkai Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4661::AID-ANIE4661>3.0.CO;2-V |
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Direct Microscopic Observation of the Time Course of Single-Molecule DNA Restriction Reactions Bürk Schäfer, Helgard Gemeinhardt, Karl Otto Greulich Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4663::AID-ANIE4663>3.0.CO;2-J |
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Extremely Long Dendronized Polymers: Synthesis, Quantification of Structure Perfection, Individualization, and SFM Manipulation Lijin Shu, A. Dieter Schlüter, Christof Ecker, Nikolai Severin, Jürgen P. Rabe Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4666::AID-ANIE4666>3.0.CO;2-1 |
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Homoaromaticity in Tris(ethylene)nickel(0) and Tris(ethyne)nickel(0) Rainer Herges, Andrea Papafilippopoulos Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4671::AID-ANIE4671>3.0.CO;2-T |
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On the Stability of Electrochemically Generated Nanoclusters - A Computer Simulation Mario G. Del Pópolo, Ezequiel P. M. Leiva, Wolfgang Schmickler Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4674::AID-ANIE4674>3.0.CO;2-B |
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Single-Compound Libraries of Organic Materials: Parallel Synthesis and Screening of Fluorescent Dyes Marc-Steffen Schiedel, Christoph A. Briehn, Peter Bäuerle Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4677::AID-ANIE4677>3.0.CO;2-U |
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Single-Compound Libraries of Organic Materials: From the Combinatorial Synthesis of Conjugated Oligomers to Structure-Property Relationships Christoph A. Briehn, Marc-Steffen Schiedel, Eva M. Bonsen, Wolfgang Schuhmann, Peter Bäuerle Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4680::AID-ANIE4680>3.0.CO;2-X |
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Temperature and Viscosity Dependence of the Spin-Directed Stereoselectivity of the Carbonyl-Alkene Photocycloaddition Axel G. Griesbeck, Samir Bondock, Murthy S. Gudipati Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4684::AID-ANIE4684>3.0.CO;2-9 |
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The Biosynthesis of Vancomycin-Type Glycopeptide Antibiotics - The Order of the Cyclization Steps Daniel Bischoff, Stefan Pelzer, Bojan Bister, Graeme J. Nicholson, Sigrid Stockert, Markus Schirle, Wolfgang Wohlleben, Günther Jung, Roderich D. Süssmuth Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4688::AID-ANIE4688>3.0.CO;2-M |
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Dimerization of Molecular Phosphorus Oxides Akbar Tellenbach, Martin Jansen Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4691::AID-ANIE4691>3.0.CO;2-P |
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Dehydrocoupling of Phosphanes Catalyzed by a Rhodium(I) Complex Volker P. W. Böhm, Maurice Brookhart Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4694::AID-ANIE4694>3.0.CO;2-7 |
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The First Dectection of Peroxo and Bis-superoxo Complexes of Aluminum: FAlO2 and FAlO4 Jan Bahlo, Hans-Jörg Himmel, Hansgeorg Schnöckel Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4696::AID-ANIE4696>3.0.CO;2-W |
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The Catalytic Enantioselective Claisen Rearrangement of an Allyl Vinyl Ether Lars Abraham, Regina Czerwonka, Martin Hiersemann Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4700::AID-ANIE4700>3.0.CO;2-6 |
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Construction of the Complete Aromatic Core of Diazonamide A by a Novel Hetero Pinacol Macrocyclization Cascade Reaction K. C. Nicolaou, Xianhai Huang, Nicolas Giuseppone, Paraselli Bheema Rao, Marco Bella, Mali V. Reddy, Scott A. Snyder Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4705::AID-ANIE4705>3.0.CO;2-D |
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Studies in the Total Synthesis of Heliquinomycinone: Proof of Concept and Assembly of a Fully Mature Spirocyclization Precursor Donghui Qin, Rex X. Ren, Tony Siu, Changsheng Zheng, Samuel J. Danishefsky Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4709::AID-ANIE4709>3.0.CO;2-Q |
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The Total Synthesis of Heliquinomycinone Tony Siu, Donghui Qin, Samuel J. Danishefsky Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4713::AID-ANIE4713>3.0.CO;2-N |
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Heat Capacity of the Mixed-Valence Complex {[(n-C3H7)4N][FeIIFeIII(dto)3]}, Phase Transition because of Electron Transfer, and a Change in Spin-State of the Whole System Tadahiro Nakamoto, Yuji Miyazaki, Miho Itoi, Yuuki Ono, Norimichi Kojima, Michio Sorai Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4716::AID-ANIE4716>3.0.CO;2-5 |
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Olefin Polymerization with [{bis(imino)pyridyl}CoIICl2]: Generation of the Active Species Involves CoI T. Martijn Kooistra, Quinten Knijnenburg, Jan M. M. Smits, Andrew D. Horton, Peter H. M. Budzelaar, Anton W Gal Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4719::AID-ANIE4719>3.0.CO;2-O |
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Design and Synthesis of a Peptide That Binds Specific DNA Sequences through Simultaneous Interaction in the Major and in the Minor Groove M. Eugenio Vázquez, Ana M. Caamaño, Jos?Martínez-Costas, Luis Castedo, Jos?L. Mascareñas Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4723::AID-ANIE4723>3.0.CO;2-L |
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Solid-Phase Capture-Release Strategy Applied to Oligosaccharide Synthesis on a Soluble Polymer Support Hiromune Ando, Shino Manabe, Yoshiaki Nakahara, Yukishige Ito Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4725::AID-ANIE4725>3.0.CO;2-9 |
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From Solutions to Surfaces: A Novel Molecular Imprinting Method Based on the Conformational Changes of Boronic-Acid-Appended Poly(L-lysine) Arianna Friggeri, Hideki Kobayashi, Seiji Shinkai,, David N. Reinhoudt Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4729::AID-ANIE4729>3.0.CO;2-M |
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Protein-Polymer Hybrid Amphiphiles Jurry M. Hannink, Jeroen J. L. M. Cornelissen, Joan A. Farrera, Philippe Foubert, Frans C. De Schryver, Nico A. J. M. Sommerdijk, Roeland J. M. Nolte Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4732::AID-ANIE4732>3.0.CO;2-P |
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A Tetrameric Nickel(II) Chair with both Antiferromagnetic Internal Coupling and Ferromagnetic Spin Alignment Vitaly V. Pavlishchuk, Sergey V. Kolotilov, Anthony W. Addison, Michael J. Prushan, Dieter Schollmeyer, Laurence K. Thompson, Eugeny A. Goreshnik Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4734::AID-ANIE4734>3.0.CO;2-D |
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A Calix[4]arene GdIII Complex Endowed with High Stability, Relaxivity, and Binding Affinity to Serum Albumin Silvio Aime, Alessandro Barge, Mauro Botta, Alessandro Casnati, Marco Fragai, Claudio Luchinat, Rocco Ungaro Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4737::AID-ANIE4737>3.0.CO;2-W |
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Li10Mg6Zn31Al3: A New Intermetallic Phase Containing Building Blocks for Decagonal Quasicrystals Chi-Shen Lee, Gordon J. Miller Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4740::AID-ANIE4740>3.0.CO;2-Z |
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Novel Coordination in the First Tellurium Porphyrin Complex: Synthesis and Crystal Structure of [Te(ttp)Cl2] Desiree S. Grubisha, Ilia A. Guzei, Najeh Al-Salim, Peter D. W. Boyd, Penelope J. Brothers, L. Keith Woo Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4743::AID-ANIE4743>3.0.CO;2-H |
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An Efficient Total Synthesis of (?-Galanthamine Catherine Guillou, Jean-Luc Beunard, Emmanuel Gras, Claude Thal Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4745::AID-ANIE4745>3.0.CO;2-5 |
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Trimerization of a Steroid Ketone To Form a Chiral Molecular Cleft Robert A. Pascal, Jr., Mary S. Mathai, Xianfeng Shen, Douglas M. Ho Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4746::AID-ANIE4746>3.0.CO;2-# |
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Recognition and Stabilization of Quadruplex DNA by a Potent New Telomerase Inhibitor: NMR Studies of the 2:1 Complex of a Pentacyclic Methylacridinium Cation with d(TTAGGGT)4 Evripidis Gavathiotis, Robert A. Heald, Malcolm F. G. Stevens, Mark S. Searle Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4749::AID-ANIE4749>3.0.CO;2-I |
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Heterolytic Cleavage of the C-C Bond of Acetonitrile with Simple Monomeric CuII Complexes: Melding Old Copper Chemistry with New Reactivity Dana S. Marlin, Marilyn M. Olmstead, Pradip K. Mascharak Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4752::AID-ANIE4752>3.0.CO;2-L |
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PtII-Catalyzed Intramolecular Reaction of Furans with Alkynes Belén Martín-Matute, Diego J. Cárdenas, Antonio M. Echavarren Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4754::AID-ANIE4754>3.0.CO;2-9 |
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Catalytic Enantioselective Isomerization of Silacyclopentene Oxides: New Strategy for Stereocontrolled Assembly of Acyclic Polyols Dong Liu, Sergey A. Kozmin Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4757::AID-ANIE4757>3.0.CO;2-S |
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The First Catalytic, Diastereoselective, and Enantioselective Crossed-Aldol Reactions of Aldehydes Scott E. Denmark, Sunil K. Ghosh Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4759::AID-ANIE4759>3.0.CO;2-G |
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Consecutive Three- and Four-Component Coupling Reactions with Anions Generated from a Butane Diacetal Desymmetrized Glycolic Acid Derivative Darren J. Dixon, Steven V. Ley, Félix Rodríguez Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4763::AID-ANIE4763>3.0.CO;2-D |
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Total Synthesis of Nominal Diazonamides - Part 1: Convergent Preparation of the Structure Proposed for (-)-Diazonamide A Jing Li, Susan Jeong, Lothar Esser, Patrick G. Harran Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4765::AID-ANIE4765>3.0.CO;2-1 |
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Total Synthesis of Nominal Diazonamides - Part 2: On the True Structure and Origin of Natural Isolates Jing Li, Anthony W. G. Burgett, Lothar Esser, Carlos Amezcua, Patrick G. Harran Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4770::AID-ANIE4770>3.0.CO;2-T |
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| Preview | ||
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Preview Published Online: 18 Dec 2001 DOI10.1002/1521-3773(20011217)40:24<4776::AID-ANIE4776>3.0.CO;2-U |